Psycho
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Psycho
I'd say with Psycho while the use of music does contribute a huge amount to the unsettling feel of the movie it seems to me more incidental music rather than a "theme tune" per se, although it has been a long time since I watched it. I think it was only using string instruments if I remember correctly?
Here's the top 25 movie themes, according to the American Film Institute:
https://en.wikipedia.org/wiki/AFI%27...of_Film_Scores
As for TV themes, I was always partial to:
https://www.youtube.com/watch?v=wL1HnDGTAK8