Miss Trunchbull
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Richard Gere as bent cop Dennis Peck in Internal Affairs
Ben Kingsley in Sexy Beast
Christopher Walken torturing Dennis Hopper in True Romance
Micheal Madsen and his ear games in Reservoir Dogs
Robert Mitchum , Robert De Niro , Cape Fear
Kathy Bates as Annie Wilkes in Misery
" I ate his liver with fava beans and a nice chianti"
Anthony Hopkins in Silence of the Lambs of course.
And Harry Lime in The Third Man was also evil underneath the charm
Dick Dastardly in Wacky Races (2013)
Dr Evil.
King Joffrey, Ramsay Bolton, The Waif, amongst others in Game of Thrones
Negan in The Walking Dead
Cruella De Ville
Very physically intimidating actor, he’s great as a malevolent force in Night of the Hunter too.
Two that have always stuck with me, both from films by David Lynch (although one a tv series as well) is Dennis Hopper in Blue Velvet and the character BOB in Twin Peaks.
Negan in The Walking Dead
He's a pussy now
Wish Maggie would just shoot him in the face which before the show went crap she would have done
This guy right here, still gives me nightmares https://www.youtube.com/watch?v=LehcJeNbFBw
Laurence Olivier as the dentist in Marathon Man - “Is it safe?”
The wicked witches, of both East and West, in the 'Wizard of Oz'.
that hit man in no country for old men
Jesus
John Doe (Kevin Spacey) in Se7en
John Malkovich in anything he’s been in.
Emperor Palpatine (Ian McDiarmid) in the Star Wars saga.